Abstract：For intensifying coupling partial oxidation and stream reforming of methane, a Nickel based catalyst was prepared with foam monolithic SiC as support. The structure of monolithic catalyst bed was optimized and the catalytic performances were investigated in a reactor with 4.8 cm height fixed bed composed of 6 block catalysts. A pilot experiment was accomplished. A bed structure consisted of multilayer catalysts was proposed for overcoming the bypass of reaction flow from the blank zoon of catalyst bed, and simultaneously bringing into the second distributing effect of oxygen. For the first time, a pilot-scale test of 200 t/a methane reforming based on this monolithic catalyst was carried out and the safety of adiabatic methane reforming technology was verified. Current research lays the foundation of further development of current technology.
Li Chunlin,Xu Hengyong,Hou Shoufu et al. Foam SiC Based Monolithic Catalyst Used for Intensifying Methane Adiabatic Reforming for Production of Syngas[J]. 化学反应工程与工艺, 2013, 29(3): 276-280.
